Springer Theses / State-to-State Dynamical Research in the F+H2 Reaction System
(Sprache: Englisch)
This book introduces a new crossed molecular beam scattering apparatus with a high time-of-flight resolution. It describes the observation of Feshbach resonances in F+H2 reaction and presents the measurement of nonadiabatic effects in F+D2 reaction.
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This book introduces a new crossed molecular beam scattering apparatus with a high time-of-flight resolution. It describes the observation of Feshbach resonances in F+H2 reaction and presents the measurement of nonadiabatic effects in F+D2 reaction.
Klappentext zu „Springer Theses / State-to-State Dynamical Research in the F+H2 Reaction System “
This thesis addresses two important and also challenging issues in the research of chemical reaction dynamics of F+H2 system. One is to probe the reaction resonance and the other is to determine the extent of the breakdown of the Born-Oppenheimer approximation (BOA) experimentally. The author introduces a state-of-the-art crossed molecular beam-scattering apparatus using a hydrogen atom Rydberg "tagging" time-of-flight method, and presents thorough state-to-state experimental studies to address the above issues. The author also describes the observation of the Feshbach resonance in the F+H2 reaction, a precise measurement of the differential cross section in the F+HD reaction, and validation of a new accurate potential energy surface with spectroscopic accuracy. Moreover, the author determines the reactivity ratio between the ground state F(2P3/2) and the excited state F*(2P1/2) in the F+D2 reaction, and exploits the breakdown of BOA in the low collision energy.
Inhaltsverzeichnis zu „Springer Theses / State-to-State Dynamical Research in the F+H2 Reaction System “
Introduction.- Hydrogen Atom Rydberg Tagging Time-of-Flight Crossed Molecular Beam Apparatus.- Dynamical Resonances in F+H2 Reactions.- The Non-Adiabatic Effects in F(2P)+D2 DF+D.
Bibliographische Angaben
- Autor: Zefeng Ren
- 2013, 2014, XII, 77 Seiten, 21 farbige Abbildungen, Masse: 15,4 x 23,7 cm, Gebunden, Englisch
- Verlag: Springer, Berlin
- ISBN-10: 3642397557
- ISBN-13: 9783642397554
Sprache:
Englisch
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